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Start-up of PN-anammox system under low inoculation quantity and its restoration after low-loading rate shock

Guoliang Zhang, Liang Zhang, Xiaoyu Han, Shujun Zhang, Yongzhen Peng

《环境科学与工程前沿（英文）》 2021年 第15卷 第2期 doi: 10.1007/s11783-020-1324-z

摘要： Abstract • PN-A was start-up under low inoculation amount and a higher NRR was achieved. • PN-anammox system was successfully restored by aggressive sludge discharge. • Increase in granular sludge was the important factor to rapid recovery. • Enrichment of AOB and AnAOB in granular sludge favors the stable operation. Partial nitritation (PN)-anaerobic ammonium oxidation (anammox) is a promising pathway for the biological treatment of wastewater. However, the destruction of the system caused by excessive accumulation of nitrate in long-term operation remains a challenge. In this study, PN-anammox was initialized with low inoculation quantity in an air-lift reactor. The nitrogen removal rate of 0.71 kgN/(m3·d) was obtained, which was far higher than the seed sludge (0.3 kgN/(m3·d)). Thereafter, excess nitrate build-up was observed under low-loading conditions, and recovery strategies for the PN-anammox system were investigated. Experimental results suggest that increasing the nitrogen loading rate as well as the concentration of free ammonium failed to effectively suppress the nitrite oxidation bacteria (NOB) after the PN-anammox system was disrupted. Afterwards, effluent back-flow was added into the reactor to control the up-flow velocity. As a result, an aggressive discharge of sludge that promoted the synergetic growth of functional bacteria was achieved, leading to the successful restoration of the PN-anammox system. The partial nitritation and anammox activity were in balance, and an increase in nitrogen removal rate up to 1.07 kgN/(m3·d) was obtained with a nitrogen removal efficiency of 82.4% after recovery. Besides, the proportion of granular sludge (over 200 mm) increased from 33.67% to 82.82%. Ammonium oxidation bacteria (AOB) along with anammox bacteria were enriched in the granular sludge during the recovery period, which was crucial for the recovery and stable operation of the PN-anammox system.

关键词： PN-anammox     Granular sludge     Excess nitrate build-up     Recovery strategy for partial nitrification     Aggressive discharge of sludge    

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Local arc discharge mechanism and requirements of power supply in micro-arc oxidation of magnesium alloy

Ming CHEN, Yuezhou MA, Yuan HAO,

《机械工程前沿（英文）》 2010年 第5卷 第1期   页码 98-105 doi: 10.1007/s11465-009-0088-8

摘要： To study the requirements of the power supply in micro-arc oxidation (MAO) of magnesium alloy, many experiments were performed under the DC, unipolar, and ambipolar pulse output modes. Based on the experimental results and electric arc theory, the separate local arc discharge mechanism was put forward. It is considered that magnesium MAO process consists of three stages including anodic oxidation, micro-arc oxidation, and large-arc discharge in turn with increasing source voltage. The MAO film is composed of metal oxides that resulted from numerous discrete local arc discharges, which accumulate the non-equilibrium structure after undergoing sudden heating and cooling cycles. Separate local arc discharge is caused by the process in which the oxygen-based gas is ionized in the conduct channel bearing electric field intensity, changed from insulator to conductor that presents sharp negative resistance effect, and produced partially high temperature to ignite locally metal oxidation. The local arc discharge model is described as four courses: gas created from electrolysis, arc discharge, metals oxidization, and cooling and shrinking of oxides. The purpose of pulse supply is to inhibit the large-arc discharge by intervening proper cooling time, which cannot be actualized by a unipolar pulse mode because of the strong capacitive load characteristics but can be reached by an ambipolar pulse supply because the negative pulse period acts as cooling time. Using a discharge loop to remove the influence of load capacitive, a new type of pulse power supply for MAO is developed, so that the large-arc problem is resolved effectively, the film-forming efficiency is improved, and the pollution of the film and electrolyte caused by negative voltage is avoided.

关键词： micro-arc oxidation     local arc discharge     pulse power supply     magnesium alloy    

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Degradation of metronidazole by dielectric barrier discharge in an aqueous solution

Zhipeng Yang, Anxing Lai, Hangyu Chen, Youxiang Yan, Ye Yang, Weiwei Zhang, Lei Wang

《环境科学与工程前沿（英文）》 2019年 第13卷 第3期 doi: 10.1007/s11783-019-1117-4

摘要：

The discharge characteristics during the degradation of MNZ by DBD were investigated.

Increasing the discharge frequency can promote the degradation of MNZ.

MNZ removal reaches 99.1% at the initial concentration of 40 ppm within 120 min.

Coexisting organic matter inhibits the degradation of MNZ.

The energy efficiency of DBD for MNZ removal is higher than other technologies.

关键词： Dielectric barrier discharge     Antibiotic     Metronidazole     Water treatment    

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Comparison between inhibitor and uncoupler for minimizing excess sludge production of an activated sludge

CHEN Guowei, XI Pengge, XU Deqian, YU Hanqing

《环境科学与工程前沿（英文）》 2007年 第1卷 第1期   页码 63-66 doi: 10.1007/s11783-007-0012-6

摘要： In order to study the minimization of excess sludge production, the reduction in the excess sludge production in the presence of an inhibitor and uncoupler was studied in this work. The experimental results show that such an addition could effectively reduce the production of excess sludge. With the energy uncoupling model established in this work, energy uncoupling coefficient () was used to evaluate the reduction in excess sludge production. The energy uncoupling coefficients in the presence of dinitrophenol (dNP), Zn, and Cu was 0.75, 0.46, and 0.18, respectively. The analysis demonstrated that energy spilling occurred in the presence of dNP, and that dNP was an effective uncoupler for reducing the production of excess activated sludge without affecting the microbial respiration activity.

关键词： uncoupling coefficient     Cu     minimization     presence     uncoupling    

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NO conversion by positive streamer discharge—effects of gas compositions and reaction conditions

HE Wei, ZHU Tianle, LI Jing

《环境科学与工程前沿（英文）》 2007年 第1卷 第2期   页码 153-158 doi: 10.1007/s11783-007-0027-z

摘要： The effects of gas compositions and reaction conditions on NO conversion by positive streamer discharge were experimentally investigated by using a link tooth wheel-cylinder reactor. The results showed that NO conversion increased w

关键词： conversion     streamer discharge     wheel-cylinder     positive streamer    

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Zero increase in peak discharge for sustainable development

Xing Fang, Junqi Li, Yongwei Gong, Xiaoning Li

《环境科学与工程前沿（英文）》 2017年 第11卷 第4期 doi: 10.1007/s11783-017-0935-5

摘要： For urban land development, some or all natural land uses (primarily pervious) are converted into impervious areas which lead to increases of runoff volume and peak discharge. Most of the developed countries require a zero increase in peak discharge for any land development, and the policy has been implemented for several decades. The policy of zero increase in peak discharge can be considered as historical and early stage for the low impact development (LID) and sustainable development, which is to maintain natural hydrological conditions by storing a part or all of additional runoff due to the development on site. The paper will discuss the policy, the policy implementation for individual projects and their impact on regional hydrology. The design rainfalls for sizing LID facilities that are determined in 206 weather stations in USA are smaller than design rainfalls for sizing detention basins. The zero-increase policy links to financial responsibility and sustainability for construction of urban stormwater infrastructures and for reducing urban flooding. The policy was compared with current practices of urban development in China to shine the light for solving urban stormwater problems. The connections and differences among LID practices, the zero-increase policy, and the flood control infrastructure were discussed. We promote and advocate the zero-increase policy on peak discharge for comprehensive stormwater management in China in addition to LID.

关键词： Stormwater management     Detention basin     Zero increase     Peak discharge     Sustainable development     Design rainfall    

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Plasma-assisted oxidation of benzoic acid

Anna Khlyustova, Nikolay Sirotkin

《化学科学与工程前沿（英文）》 2020年 第14卷 第4期   页码 513-521 doi: 10.1007/s11705-019-1825-0

摘要： Plasma-assisted oxidation of organic compounds is one of the developing technologies for wastewater treatment. Plasmas effectively accelerate degradation processes due to plasma generated reactive species and ultra-violet radiation. Oxidation of benzoic acid in aqueous solutions by the atmospheric pressure glow discharge and underwater diaphragm discharge was studied and monitored by fluorescence and spectrophotometric methods. Discharge type and solution pH affect the formation rates of mono- and dihydroxybenzoic acids. Dihydroxyl derivatives were formed only by glow discharge action. The yields of hydroxyl radical were estimated on the kinetics data for the hydroxylation of benzoic acid. The steps of the hydroxylation processes and further oxidation were described.

关键词： atmospheric pressure glow discharge     underwater diaphragm discharge     oxidation     benzoic acid     hydroxyl radical    

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Co-pyrolysis of sludge and kaolin/zeolite in a rotary kiln: Analysis of stabilizing heavy metals

《环境科学与工程前沿（英文）》 2022年 第16卷 第7期 doi: 10.1007/s11783-021-1488-1

摘要：

• Adding kaolin/zeolite promotes the formation of stable heavy metals.

关键词： Co-pyrolysis     Sewage sludge     Heavy metals     Rotary kiln     Immobilization mechanism    

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Cultivation of aerobic granular sludge in a conventional, continuous flow, completely mixed activatedsludge system

Xi CHEN,Linjiang YUAN,Wenjuan LU,Yuyou LI,Pei LIU,Kun NIE

《环境科学与工程前沿（英文）》 2015年 第9卷 第2期   页码 324-333 doi: 10.1007/s11783-014-0627-3

摘要： Aerobic granules were formed in a conventional, continuous flow, completely mixed activated sludge system (CMAS). The reactor was inoculated with seed sludge containing few filaments and fed with synthetic municipal wastewater. The settling time of the sludge and the average dissolved oxygen (DO) of the reactor were 2 h and 4.2 mg·L , respectively. The reactor was agitated by a stirrer, with a speed of 250 r·min , to ensure good mixing．The granular sludge had good settleability, and the sludge volume index (SVI) was between 50 and 90 mL·g . The laser particle analyzer showed the diameter of the granules to be between 0.18 and 1.25 mm. A scanning electron microscope (SEM) investigation revealed the predominance of sphere-like and rod-like bacteria, and only few filaments grew in the granules. The microbial community structure of the granules was also analyzed by polymerase chain reaction-denaturing gradient gel electrophoresis (PCR-DGGE). Sequencing analysis indicated the dominant species were α, β, and γ- , , and . The data from the study suggested that aerobic granules could form, if provided with sufficient number of filaments and high shear force. It was also observed that a high height-to-diameter ratio of the reactor and short settling time were not essential for the formation of aerobic granular sludge.

关键词： aerobic granular sludge     completely mixed activated sludge system (CMAS)     continuous flow     shear force     filamentous bacteria     polymerase chain reaction-denaturing gradient gel electrophoresis (PCR-DGGE)    

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Conversion of methane through dielectric-barrier discharge plasma

WANG Baowei, CAO Xiaolei, YANG Kuanhui, XU Genhui

《化学科学与工程前沿（英文）》 2008年 第2卷 第4期   页码 373-378 doi: 10.1007/s11705-008-0070-8

摘要： Methane coupling to produce C hydrocarbons through a dielectric-barrier discharge (DBD) plasma reaction was studied in four DBD reactors. The effects of high voltage electrode position, different discharge gap, types of inner electrode, volume ratio of hydrogen to methane and air cooling method on the conversion of methane and distribution of products were investigated. Conversion of methane is obviously lower when a high voltage electrode acts as an outer electrode than when it acts as an inner electrode. The lifting of reaction temperature becomes slow due to cooling of outer electrode and the temperature can be controlled in the expected range of 60°C–150°C for ensuring better methane conversion and safe operation. The parameters of reactors have obvious effects on methane conversion, but it only slightly affects distribution of the products. The main products are ethylene, ethane and propane. The selectivity of C hydrocarbons can reach 74.50% when volume ratio of hydrogen to methane is 1.50.
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Control of sludge settleability and nitrogen removal under low dissolved oxygen condition

Zhaoxu PENG, Yongzhen PENG, Zhenbo YU, Xuliang LIU, Xiaoling LI, Randeng WANG

《环境科学与工程前沿（英文）》 2012年 第6卷 第6期   页码 884-891 doi: 10.1007/s11783-012-0408-9

摘要： Low dissolved oxygen (DO) is an energy-saving condition in activated sludge process. To investigate the possible application of limited filamentous bulking (LFB) in sequencing batch reactor (SBR), two lab-scale SBRs were used to treat synthetic domestic wastewater and real municipal wastewater, respectively. The results showed that prolonging low DO aeration duration and setting pre-anoxic (anaerobic) phase were effective strategies to induce and inhibit filamentous sludge bulking, respectively. According to the sludge settleability, LFB could be maintained steadily by adjusting operation patterns. Filamentous bacteria content and sludge volume index (SVI) were likely correlated. SVI fluctuated dramatically within a few cycles when around 200 mL·g , where altering operation pattern could change sludge settleability in spite of the unstable status of activated sludge system. Energy consumption by aeration reduced under low DO LFB condition, whereas the nitrification performance deteriorated. However, short-cut nitrification and simultaneous nitrification denitrification (SND) were prone to take place under such conditions. When the cycle time kept constant, the anoxic (anaerobic) to aerobic time ratio was determining factor to the SND efficiency. Similarity keeping aerobic time as constant, the variation trends of SND efficiency and specific SND rate were uniform. SBR is a promising reactor to apply the LFB process in practice.

关键词： limited filamentous bulking     sequencing batch reactor     sludge settleability     sludge volume index     simultaneous nitrification denitrification    

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Liquid discharge plasma for fast biomass liquefaction at mild conditions: The effects of homogeneous

Sen Wang, Shiyun Liu, Danhua Mei, Rusen Zhou, Congcong Jiang, Xianhui Zhang, Zhi Fang, Kostya (Ken) Ostrikov

《化学科学与工程前沿（英文）》 2020年 第14卷 第5期   页码 763-771 doi: 10.1007/s11705-019-1896-y

摘要： Non-thermal plasma exhibits unique advantages in biomass conversion for the sustainable production of higher-value energy carriers. Different homogeneous catalysts are usually required for plasma-enabled biomass liquefaction to achieve time-and energy-efficient conversions. However, the effects of such catalysts on the plasma-assisted liquefaction process and of the plasma on those catalysts have not been thoroughly studied. In this study, an electrical discharge plasma is employed to promote the direct liquefaction of sawdust in a mixture of polyethylene glycol 200 and glycerol. Three commonly used chemicals, sulfuric acid, nitric acid and sodium -toluene sulfate, were selected as catalysts. The effects of the type of catalyst and concentration on the liquefaction yield were examined; further, the roles of the catalysts in the plasma liquefaction process have been discussed. The results showed that the liquefaction yield attains a value of 90% within 5 min when 1% sulfuric acid was employed as the catalyst. Compared with the other catalysts, sulfuric acid presents the highest efficiency for the liquefaction of sawdust. It was observed that hydrogen ions from the catalyst were primarily responsible for the significant thermal effects on the liquefaction system and the generation of large quantities of active species; these effects directly contributed to a higher efficacy of the plasma-enabled liquefaction process.

关键词： discharge plasma     biomass liquefaction     catalyst     homogeneous catalysts    

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High-solid anaerobic digestion of sewage sludge: achievements and perspectives

《环境科学与工程前沿（英文）》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1364-4

摘要：

• High-solid anaerobic digestion (HS-AD) of sewage sludge (SS) is overviewed.

关键词： High-solid effect     Anaerobic fermentation     Methane production     Biodegradability     Sludge treatment    

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A review on sustainable reuse applications of Fenton sludge during wastewater treatment

《环境科学与工程前沿（英文）》 2022年 第16卷 第6期 doi: 10.1007/s11783-021-1511-6

摘要：

• The sustainable approaches related to Fenton sludge reuse systems are summarized.

关键词： Fenton sludge     Heavy metals     Coagulant     Iron source     Heterogeneous catalyst    

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Properties and effect of forming sewage sludge into lightweight ceramics

Min YUE, Qinyan YUE, Yuanfeng QI, Baoyu GAO, Hui YU

《环境科学与工程前沿（英文）》 2012年 第6卷 第1期   页码 117-124 doi: 10.1007/s11783-010-0220-3

摘要： In this work we investigated the chemical, thermal and toxic properties of dried sewage sludge (DSS), the preparation and properties of lightweight sludge ceramic (LSC) and the mechanisms of action of the organic and inorganic foaming agents (OFAs and IFAs). The chemical components and thermal properties of the raw materials were studied by Energy Dispersive X-ray Detection (EDX) and Thermogravimetric Analysis and Differential Scanning Calorimetry (DSC/TGA). The mineral phases of the raw materials and the formed ceramics were determined by X-ray Diffraction (XRD). The leaching characteristics of heavy metals were investigated with Inductively Coupled Plasma Atomic Emission Spectrometry (ICP-AES). Different ratios of DSS and clay were mixed and pressed into raw pellets. After drying and preheating treatment, the raw pellets were sintered at 1150°C for 10 min. The physical properties of LSC (50 wt% DSS added) were tested. The results showed that when the addition of DSS was above 50 wt%, LSC began to shrink, and a maximum density occurred. The environmental safety of LSC was satisfactory. XRD showed that some new mineral phases formed in the LSC. Observation of the microstructure by Scanning Electron Microscope (SEM) indicated that the body of LSC was porous.

关键词： sludge     foaming agents     ceramics     preheating process    

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标题 作者 时间 类型 操作

Start-up of PN-anammox system under low inoculation quantity and its restoration after low-loading rate shock

Guoliang Zhang, Liang Zhang, Xiaoyu Han, Shujun Zhang, Yongzhen Peng

期刊论文

Local arc discharge mechanism and requirements of power supply in micro-arc oxidation of magnesium alloy

Ming CHEN, Yuezhou MA, Yuan HAO,

期刊论文

Degradation of metronidazole by dielectric barrier discharge in an aqueous solution

Zhipeng Yang, Anxing Lai, Hangyu Chen, Youxiang Yan, Ye Yang, Weiwei Zhang, Lei Wang

期刊论文

Comparison between inhibitor and uncoupler for minimizing excess sludge production of an activated sludge

CHEN Guowei, XI Pengge, XU Deqian, YU Hanqing

期刊论文

NO conversion by positive streamer discharge—effects of gas compositions and reaction conditions

HE Wei, ZHU Tianle, LI Jing

期刊论文

Zero increase in peak discharge for sustainable development

Xing Fang, Junqi Li, Yongwei Gong, Xiaoning Li

期刊论文

Plasma-assisted oxidation of benzoic acid

Anna Khlyustova, Nikolay Sirotkin

期刊论文

Co-pyrolysis of sludge and kaolin/zeolite in a rotary kiln: Analysis of stabilizing heavy metals

期刊论文

Cultivation of aerobic granular sludge in a conventional, continuous flow, completely mixed activatedsludge system

Xi CHEN,Linjiang YUAN,Wenjuan LU,Yuyou LI,Pei LIU,Kun NIE

期刊论文

Conversion of methane through dielectric-barrier discharge plasma

WANG Baowei, CAO Xiaolei, YANG Kuanhui, XU Genhui

期刊论文

Control of sludge settleability and nitrogen removal under low dissolved oxygen condition

Zhaoxu PENG, Yongzhen PENG, Zhenbo YU, Xuliang LIU, Xiaoling LI, Randeng WANG

期刊论文

Liquid discharge plasma for fast biomass liquefaction at mild conditions: The effects of homogeneous

Sen Wang, Shiyun Liu, Danhua Mei, Rusen Zhou, Congcong Jiang, Xianhui Zhang, Zhi Fang, Kostya (Ken) Ostrikov

期刊论文

High-solid anaerobic digestion of sewage sludge: achievements and perspectives

期刊论文

A review on sustainable reuse applications of Fenton sludge during wastewater treatment

期刊论文

Properties and effect of forming sewage sludge into lightweight ceramics

Min YUE, Qinyan YUE, Yuanfeng QI, Baoyu GAO, Hui YU

期刊论文